REVIEW OF EVALUATIONS FOR THE TITANIUM ISOTOPES

 

 

INTRODUCTION

 

Systematic comparison with experimental data from EXFOR was made with the ENDVER package for the following evaluations:

            ENDF/B-VII.1   http://www.nndc.bnl.gov/

            JEFF-3.1.2         http://www-nds.iaea.org/exfor/endf.htm

            JEFF-3.2T          http://www.oecd-nea.org/dbdata/jeff-beta/JEFF32T1

            JENDL-4.0        http://www-nds.iaea.org/exfor/endf.htm

 

The comparisons are presented for the natural element, which has the most abundant database of experimental data, although similar plots exist for individual isotopes.

 

All isotopes of titanium from each library were processed with the PrePro-2010 codes and additional codes from the ENDVER package for plotting purposes.


Detailed graphical comparison can be viewed from nTi-0.htm; plot numbers in the text below refer to this list. The plots in the list can be viewed in the interactive mode. The plots in the discussion below have been converted to "gif" for the convenience of the users.

 

NOTE:

To view the plots interactively it is necessary to download the ZVView code and associate ZVD files with this application.

 

 

CROSS SECTIONS

 

The cross sections are generally in good agreement with measurements. Specific conclusions can be summarised as follows below. In the JEFF-3.2T library some of the isotopes are evaluated only up to 20 MeV, therefore the comparisons above this energy are meaningless.


The total cross sections from JEFF-3.2T seems to agree best with available experimental data in the EXFOR database, particularly in the resonance region, as well as at higher energies between 6 MeV and 12 MeV.


Considering the scatter in the measured inelastic cross sections data, all evaluations show fairly good consistency.


Very few measurements exist for the capture cross section. The strong dip in the cross section below the first resonance in JEFF-3.2T might be unphysical. It is not present in the ENDF/B-VII.1 library.


The proton-production cross sections from all evaluated libraries are much higher than the single measurement of Hassler (1962), which is old.


The tritium-production cross sections in ENDF/B-VII.1 and JENDL-4.0 are identical and lower than the single measurement by Biro (1975). The JEFF-3.2T cross sections are higher, but with uncertainties that enclose the measurement.

 

The alpha-production cross section in JEFF-3.2T has some structure and is assigned a very small uncertainty below 15 MeV, which is inconsistent with the two measurements by Takagi (1986) and by Kneff (1986). Overall, the cross sections in all libraries are comparable.

The 46V production cross sections are in good agreement in all libraries with the measurements by Greenwood (1987). The single point measured by Meadows (1987) at 14.85 MeV is lower by more than the uncertainty interval.

The 47V production cross sections in JEFF-3.2T tend to follow the data by Greenwood (1987). The measurements by Molla (1991) are higher, while the single-point measurement by Meadows (1987) is lower. The ENDF/B-VII.1 cross section curve is considerably lower.

All evaluations predict the 48V production cross sections close to the measurement by Meadows (1987), which is significantly lower than the measurement by Molla (1991) .


The average cosing of scattering (mu-bar, reconstructed from the angular distributions) in ENDF/B-VII.1 around 1 MeV follows closely the structure in the measured data, while all other evaluations predict a smooth behaviour.

 

ANGULAR DISTRIBUTIONS

 

At low energies (from about 0.3 MeV) there are considerable differences between the evaluation, which gradually decrease as the incident neutron energy increases (e.g. 1.5 MeV). At 2 MeV and above the agreement between the data in the libraries with measured data is quite good. At energies above 7 MeV one has to be careful about the interpretation of experimental measurements due to possible contamination of the elastic angular distributions with the inelastic contribution.

 

NEUTRON EMISSION SPECTRA

 

The angle-integrated neutron emission spectra in the JEFF-3.2T are in excellent agreement with the measured data by Schmidt (2006), which span from 7.9 MeV to 14.6 MeV. Good agreement is observed at intermediate energies (e.g. 10.2 MeV). A few measurements are available from other authors. Experimental data at 14.1 MeV are particularly abundant.



PROTON EMISSION SPECTRA


Angle-integrated proton emission spectrum at 14.1 MeV was measured by Takagi (2000). The spectrum extracted from JEFF-3.2T is much lower. Other libraries do not contain spectral information for protons.

 

ALPHA EMISSION SPECTRA

 

Angle-integrated alpha emission spectrum at 14.1 MeV was measured by Takagi (2000). The spectrum extracted from JEFF-3.2T is of approximately the same magnitude, but different in shape. Other libraries do not contain spectral information for alpha particles.


GAMMA EMISSION SPECTRA

 

The gamma-emission spectrum from the radiative capture reaction measured by Voignier (1992) agrees well with the data from the ENDF/B-VII.1 library, which includes detailed structure from the discrete gamma lines. The gamma spectrumin the JEFF-3.2T library in the MeV region is much lower and without detailed structure.